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Ethylene glycol-mediated rapid synthesis of carbon-coated ZnFe2O4 nanoflakes with long-term and high-rate performance for lithium-ion batteries EI SCIE PubMed Scopus
期刊论文 | 2018 , 47 (10) , 3521-3529 | DALTON TRANSACTIONS
WoS CC Cited Count: 4
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Abstract :

Carbonaceous hybrid nanocomposites with a porous flaky structure hold great promise as high-performance electrodes for lithium-ion batteries (LIBs); yet large-scale synthesis is still a challenge. In this work, we successfully develop a novel carbon hybrid structure of carbon-coated ZnFe2O4 nanoflakes (ZnFe2O4@C NFs) through a fast ethylene glycol (EG)-mediated metal alkoxide method, refluxing at 200 degrees C in EG and a post-calcination at 500 degrees C in a N-2 atmosphere. The organic components in the pre-synthesized ZnFe-alkoxide precursor (ZnFe2(OCH2CH2O)(4)) can be transferred into an amorphous carbon layer easily surrounding the crystalline ZnFe2O4 subunits during the annealing process. The flaky mor-phologies of the as-prepared ZnFe2O4@C hybrids are highly dependent on the refluxing temperature. Upon increasing the refluxing temperature from 140 degrees C to 200 degrees C, the sphere-like morphology of the ZnFe2O4@C composites gradually evolves into microflowers and separate nanoflakes. When used as an anode for LIBs, the hybrid ZnFe2O4@C NFs present excellent electrochemical performance with high discharge capacity, long-term cyclic stability and superior high-rate capability. Even after 1000 cycles at 0.5 A g(-1), the hybrid ZnFe2O4@C NFs still deliver a stable reversible discharge capacity of 778.6 mA h g(-1).

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GB/T 7714 Gao, Guoxin , Shi, Lei , Lu, Shiyao et al. Ethylene glycol-mediated rapid synthesis of carbon-coated ZnFe2O4 nanoflakes with long-term and high-rate performance for lithium-ion batteries [J]. | DALTON TRANSACTIONS , 2018 , 47 (10) : 3521-3529 .
MLA Gao, Guoxin et al. "Ethylene glycol-mediated rapid synthesis of carbon-coated ZnFe2O4 nanoflakes with long-term and high-rate performance for lithium-ion batteries" . | DALTON TRANSACTIONS 47 . 10 (2018) : 3521-3529 .
APA Gao, Guoxin , Shi, Lei , Lu, Shiyao , Gao, Ting , Li, Zhaoyang , Gao, Yiyang et al. Ethylene glycol-mediated rapid synthesis of carbon-coated ZnFe2O4 nanoflakes with long-term and high-rate performance for lithium-ion batteries . | DALTON TRANSACTIONS , 2018 , 47 (10) , 3521-3529 .
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Red blood cell-like hollow carbon sphere anchored ultrathin Na2Ti3O7 nanosheets as long cycling and high rate-performance anodes for sodium-ion batteries EI SCIE Scopus
期刊论文 | 2018 , 6 (27) , 13164-13170 | JOURNAL OF MATERIALS CHEMISTRY A
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Abstract :

Sodium titanate (Na2Ti3O7) has been proved to be a potential anode material for sodium-ion batteries. However, its poor rate capability and low electrical conductivity has seriously hindered its application. Therefore, a unique red blood cell-like hollow carbon sphere supported Na2Ti3O7 sodium titanate nanosheet structure (Na2Ti3O7@RHCS) was designed here, which can both improve the electrical conductivity and preserve the structural stability, thus obtaining high rate performance. In addition, the red blood cell-like spherical structure can greatly increase the compacted density via a dense packing mode just like red blood cells stacked together one by one. Meanwhile, the ultrathin nanosheet-like morphology of Na2Ti3O7 could further increase the number of active reaction sites and reduce the diffusion path of sodium ions during the charge-discharge process. This well-designed material exhibits a good cycling performance: a reversible capacity of 110.46 mA h g(-1) at 5C and 45.71 mA h g(-1) at 50C.

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GB/T 7714 Chen, Sheng , Pang, Yuanchao , Liang, Jin et al. Red blood cell-like hollow carbon sphere anchored ultrathin Na2Ti3O7 nanosheets as long cycling and high rate-performance anodes for sodium-ion batteries [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2018 , 6 (27) : 13164-13170 .
MLA Chen, Sheng et al. "Red blood cell-like hollow carbon sphere anchored ultrathin Na2Ti3O7 nanosheets as long cycling and high rate-performance anodes for sodium-ion batteries" . | JOURNAL OF MATERIALS CHEMISTRY A 6 . 27 (2018) : 13164-13170 .
APA Chen, Sheng , Pang, Yuanchao , Liang, Jin , Ding, Shujiang . Red blood cell-like hollow carbon sphere anchored ultrathin Na2Ti3O7 nanosheets as long cycling and high rate-performance anodes for sodium-ion batteries . | JOURNAL OF MATERIALS CHEMISTRY A , 2018 , 6 (27) , 13164-13170 .
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Facile synthesis of ultrathin and perpendicular NiMn2O4 nanosheets on reduced graphene oxide as advanced electrodes for supercapacitors EI SCIE Scopus
期刊论文 | 2018 , 5 (7) , 1714-1720 | INORGANIC CHEMISTRY FRONTIERS
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Ultrathin nickel manganese oxide nanosheets grown vertically on reduced graphene oxide (NiMn2O4 NSs@rGO) were successfully fabricated through a facile co-precipitation and thermal treatment process. Such a unique nanostructure can not only facilitate electron transfer and electrolyte penetration but also withstand the structural damage of the active materials in electrochemical reactions. The resulting product NiMn2O4 NSs@rGO was characterized by X-ray diffraction (XRD), field emission scanning electron microscopy (FESEM), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS) and Brunauer-Emmett-Teller (BET) analysis. When evaluated for its potential as an electrode material in supercapacitors, the as-synthesized NiMn2O4 NSs@rGO nanocomposite exhibits enhanced energy storage performance with high specific capacitance (1243 F g(-1) at 3 A g(-1)) and prominent cycle life (80.8% capacitance retention after 5000 cycles). These results indicate that the ultrathin and perpendicular NiMn2O4 nanosheets with rGO substrates obtained from this green and facile route hold great prospects in high performance supercapacitor applications.

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GB/T 7714 Li, Long , Hu, Hongli , Ding, Shujiang . Facile synthesis of ultrathin and perpendicular NiMn2O4 nanosheets on reduced graphene oxide as advanced electrodes for supercapacitors [J]. | INORGANIC CHEMISTRY FRONTIERS , 2018 , 5 (7) : 1714-1720 .
MLA Li, Long et al. "Facile synthesis of ultrathin and perpendicular NiMn2O4 nanosheets on reduced graphene oxide as advanced electrodes for supercapacitors" . | INORGANIC CHEMISTRY FRONTIERS 5 . 7 (2018) : 1714-1720 .
APA Li, Long , Hu, Hongli , Ding, Shujiang . Facile synthesis of ultrathin and perpendicular NiMn2O4 nanosheets on reduced graphene oxide as advanced electrodes for supercapacitors . | INORGANIC CHEMISTRY FRONTIERS , 2018 , 5 (7) , 1714-1720 .
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Self-assembly of Fe2O3/ordered mesoporous carbons for high-performance lithium-ion batteries EI SCIE Scopus
期刊论文 | 2018 , 817 , 65-72 | JOURNAL OF ELECTROANALYTICAL CHEMISTRY
WoS CC Cited Count: 1 SCOPUS Cited Count: 2
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Abstract :

Fe2O3/ordered mesoporous carbons (OMCs) have been synthesized by a facile one-pot hydrothermal method via self-assembly process. The combination of OMCs and anchored Fe2O3 nanoparticles shows a synergistic effect which results in a kind of anode materials with enhanced electrochemical performance for lithium ion batteries. OMCs with highly porous mesostructure and good conductivity not only alleviate the problem of volume variation and agglomeration of Fe2O3, but shorten the diffusion pathway of Li+ ions, which efficiently overcomes the problem of rapid capacity loss of iron oxide. Moreover, appropriate loading amount of Fe2O3 nanoparticles is believed to be a key factor to enhance the capacity of anode materials. The materials deliver an excellent reversible capacity of 789 mAh g(-1 )at a current density of 100 mA g(-1) after 120 cycles.

Keyword :

Fe2O3 Lithium-ion battery Self-assembly Ordered mesoporous carbon

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GB/T 7714 Kang, Liying , Yang, Zhenglong , Xu, Yanbin et al. Self-assembly of Fe2O3/ordered mesoporous carbons for high-performance lithium-ion batteries [J]. | JOURNAL OF ELECTROANALYTICAL CHEMISTRY , 2018 , 817 : 65-72 .
MLA Kang, Liying et al. "Self-assembly of Fe2O3/ordered mesoporous carbons for high-performance lithium-ion batteries" . | JOURNAL OF ELECTROANALYTICAL CHEMISTRY 817 (2018) : 65-72 .
APA Kang, Liying , Yang, Zhenglong , Xu, Yanbin , Jiang, Wei , Wang, Feng , Meng, Yanfeng et al. Self-assembly of Fe2O3/ordered mesoporous carbons for high-performance lithium-ion batteries . | JOURNAL OF ELECTROANALYTICAL CHEMISTRY , 2018 , 817 , 65-72 .
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Microwave-assisted fast synthesis of hierarchical NiCo2O4 nanoflower-like supported Ni(OH)(2) nanoparticles with an enhanced electrocatalytic activity towards methanol oxidation EI SCIE Scopus
期刊论文 | 2018 , 5 (1) , 172-182 | INORGANIC CHEMISTRY FRONTIERS
WoS CC Cited Count: 2 SCOPUS Cited Count: 3
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Abstract :

NiCo2O4 nanoflowers were synthesized through a microwave-assisted hydrothermal method and used as a type support for Ni(OH)(2) nanoparticles. In the three-dimensional NiCo2O4 nanoflowers, twodimensional ultrathin nanosheets supported the Ni(OH)(2) nanoparticles by homogeneous precipitation. The materials were characterized by field-emission scanning electron microscopy, transmission electron microscopy, X-ray photoelectron spectroscopy, and Raman spectroscopy. The electrochemical oxidation of methanol was probed through the NiCo2O4/Ni(OH)(2) modification on a glassy carbon electrode in an alkaline medium by employing cyclic voltammetry (CV) and chronoamperometry (CA). The current density of the NiCo2O4/ Ni(OH)(2) electrode in 1 M KOH with 0.5 M methanol ascends to 92.3 A g(-1) and restores to 94.6% of the primitive value through the replacement with a new solution after a long-term CV cycling (500 cycles). Therefore, the compounds further corroborate their excellent electrocatalytic activity and superb perennial stability for methanol oxidation. This study demonstrates that NiCo2O4/ Ni(OH)(2) is a peculiar material with an outstanding performance in direct methanol fuel cells.

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GB/T 7714 Wang, Bingrong , Cao, Yang , Chen, Yong et al. Microwave-assisted fast synthesis of hierarchical NiCo2O4 nanoflower-like supported Ni(OH)(2) nanoparticles with an enhanced electrocatalytic activity towards methanol oxidation [J]. | INORGANIC CHEMISTRY FRONTIERS , 2018 , 5 (1) : 172-182 .
MLA Wang, Bingrong et al. "Microwave-assisted fast synthesis of hierarchical NiCo2O4 nanoflower-like supported Ni(OH)(2) nanoparticles with an enhanced electrocatalytic activity towards methanol oxidation" . | INORGANIC CHEMISTRY FRONTIERS 5 . 1 (2018) : 172-182 .
APA Wang, Bingrong , Cao, Yang , Chen, Yong , Wang, Ruzhi , Wang, Xiaohong , Lai, Xiaoyong et al. Microwave-assisted fast synthesis of hierarchical NiCo2O4 nanoflower-like supported Ni(OH)(2) nanoparticles with an enhanced electrocatalytic activity towards methanol oxidation . | INORGANIC CHEMISTRY FRONTIERS , 2018 , 5 (1) , 172-182 .
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Hierarchical micro/mesoporous nitrogen-doped carbons derived from hypercrosslinked polymers for highly efficient oxygen reduction reaction EI SCIE Scopus
期刊论文 | 2018 , 138 , 348-356 | CARBON
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Abstract :

Exploring highly efficient non-Pt oxygen reduction reaction (ORR) electrocatalysts is an inevitable trend in the progress of various sustainable energy storage and conversion technologies. Herein, we prepare three kinds of hierarchical porous carbons, derived from hypercrosslinked polyaniline (HCP-An), polypyrrole (HCP-Py) and polymethylbenzene (HCP-MB) through a facile Friedel-Crafts reaction, among which NPC-An-900 exhibits outstanding ORR catalytic performance combining high surface area, good conductivity and high nitrogen-doped content. The hypercrosslinked polyaniline ensures micro-/mesoporous skeleton and prevents collapse during the pyrolysis process for NPC-An-900 with a high surface area of 2938.31 m(2) g(-1) and hierarchical micro-/mesoporous structure (1-8 nm). High nitrogen-doping content of NCP-An-900 is up to 7.02 at.% with pyridinic N as the main nitrogen doped type of 48.5% of the total nitrogen content. NPC-An-900 manifests an onset potential of 0.96 V (vs. RHE) with a high limiting current density of -5.31 mA cm(-2) (superior to the commercial Pt/C of -5.20 mA cm(-2)) and excellent stability with current retention of 96.2% over 7.5 h. Furthermore, the extraordinary tolerance against methanol corrosion would also indicate its potential practical applications. This simple and universal synthesis strategy can be widely applied in the preparation of other porous heteroatom-doped carbons derived functional polymers towards energy storage and conversion. (C) 2018 Elsevier Ltd. All rights reserved.

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GB/T 7714 Xu, Jingjing , Shi, Lei , Wang, Jianan et al. Hierarchical micro/mesoporous nitrogen-doped carbons derived from hypercrosslinked polymers for highly efficient oxygen reduction reaction [J]. | CARBON , 2018 , 138 : 348-356 .
MLA Xu, Jingjing et al. "Hierarchical micro/mesoporous nitrogen-doped carbons derived from hypercrosslinked polymers for highly efficient oxygen reduction reaction" . | CARBON 138 (2018) : 348-356 .
APA Xu, Jingjing , Shi, Lei , Wang, Jianan , Lu, Shiyao , Wang, Yuankun , Gao, Guoxin et al. Hierarchical micro/mesoporous nitrogen-doped carbons derived from hypercrosslinked polymers for highly efficient oxygen reduction reaction . | CARBON , 2018 , 138 , 348-356 .
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A Highly Efficient Electrocatalyst Derived from Polyaniline@CNTs-SPS** for the Oxygen Reduction Reaction EI SCIE Scopus
期刊论文 | 2018 , 5 (1) , 195-200 | CHEMELECTROCHEM
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Abstract :

It is of vital importance to develop novel, low-cost, and high-efficiency electrocatalysts for the oxygen reduction reaction (ORR), which have a considerable impact on electrochemical energy conversion and storage devices, such as fuel cells and metal-air batteries. In this work, we demonstrate highly active nitrogen-doped carbons with uniform hierarchical structures through sulfonated polystyrene (SPS), regulating the distribution of the PANI covering on carbon nanotubes (CNTs), prepared by using a reliable and controllable route. The as-prepared electrocatalyst shows outstanding activity towards the ORR in alkaline media, manifesting comparable or even better performance compared to commercial Pt/C. The optimized nitrogen-doped CNTs exhibit an onset potential (E-onset) of 0.94 V (vs. reversible hydrogen electrode (RHE)) and half-wave potential (E-1/2) of 0.83 V (vs. RHE) in 0.1 M KOH with superior stability, durability, and methanol tolerance, suggesting their promising applications in fuel cells and metal-air batteries. The significantly improved electrochemical properties demonstrate that the unique SPS layer anchoring on the surface of CNTs in the as-designed PANI@CNTs-SPS contributes to a uniform distribution of nitrogen sites throughout the catalyst.

Keyword :

oxygen reduction reaction PANI nitrogen-doped carbon carbon nanotubes electrocatalyst

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GB/T 7714 Xu, Jingjing , Lu, Shiyao , Zhou, Han et al. A Highly Efficient Electrocatalyst Derived from Polyaniline@CNTs-SPS** for the Oxygen Reduction Reaction [J]. | CHEMELECTROCHEM , 2018 , 5 (1) : 195-200 .
MLA Xu, Jingjing et al. "A Highly Efficient Electrocatalyst Derived from Polyaniline@CNTs-SPS** for the Oxygen Reduction Reaction" . | CHEMELECTROCHEM 5 . 1 (2018) : 195-200 .
APA Xu, Jingjing , Lu, Shiyao , Zhou, Han , Chen, Xu , Wang, Yuankun , Xiao, Chunhui et al. A Highly Efficient Electrocatalyst Derived from Polyaniline@CNTs-SPS** for the Oxygen Reduction Reaction . | CHEMELECTROCHEM , 2018 , 5 (1) , 195-200 .
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Dielectric gels with ultra-high dielectric constant, low elastic modulus, and excellent transparency EI Scopus SCIE
期刊论文 | 2018 , 10 , 821-826 | NPG Asia Materials
WoS CC Cited Count: 1 SCOPUS Cited Count: 1
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We designed dielectric gels, a new type of polymer-based dielectric material. By using solvents with high dielectric constants, the gels achieve a unique combination of ultra-high dielectric constant, low elastic modulus, and excellent transparency, which are extremely challenging or impossible to realize with traditional polymer dielectrics. The gels exhibit high stretchability (stretch of approximately 10) and low mechanical hysteresis. We demonstrated the use of the dielectric gels by fabricating a bioinspired tunable lens, the focal length of which can be adjusted by varying the applied voltage. We believe that the dielectric gels, as a new type of polymer dielectric, offer new opportunities for soft robotics, sensors, electronics, optics, and biomimetics. © 2018, The Author(s).

Keyword :

Applied voltages Focal lengths High dielectric constants Low elastic modulus Mechanical hysteresis Polymer dielectrics Soft robotics Ultra-high dielectric constant

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GB/T 7714 Shi, Lei , Yang, Ruisen , Lu, Shiyao et al. Dielectric gels with ultra-high dielectric constant, low elastic modulus, and excellent transparency [J]. | NPG Asia Materials , 2018 , 10 : 821-826 .
MLA Shi, Lei et al. "Dielectric gels with ultra-high dielectric constant, low elastic modulus, and excellent transparency" . | NPG Asia Materials 10 (2018) : 821-826 .
APA Shi, Lei , Yang, Ruisen , Lu, Shiyao , Jia, Kun , Xiao, Chunhui , Lu, Tongqing et al. Dielectric gels with ultra-high dielectric constant, low elastic modulus, and excellent transparency . | NPG Asia Materials , 2018 , 10 , 821-826 .
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New Theoretical Strategy for the Correlation of Oxygen Evolution Performance and Metal Catalysts Adsorption at BiVO4 Surfaces EI Scopus SCIE
期刊论文 | 2018 , 122 (44) , 25195-25203 | Journal of Physical Chemistry C
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© 2018 American Chemical Society. The oxygen evolution reaction (OER) is the limiting process in photoelectrochemical water splitting. Bismuth vanadate (BiVO4) is a very promising photoanode material for this but suffers experimentally from poor catalytic performance for OER. Here, we theoretically explored, by means of density functional theory calculations, supporting single metal atoms (i.e., Ag, Au, Pd, and Pt) as an effective strategy to enhance the catalytic activity of BiVO4. The OER performance of different surfaces was evaluated with the intermediate adsorption energies from a thermodynamic viewpoint. The electronic structure study was employed in details to comprehend the adsorption-changing mechanism. Based on the results, several linear relationships were derived among the adsorption energies of reaction intermediates in this work, and a volcano plot was presented to unravel the theoretical activities over different BiVO4 surfaces. It was found that the metal center dominated the interaction with the intermediates and the substrate played an instrumental role in achieving a qualified energy-level matching requirement for bonding. A new method for calculating the d-band center of singe-metal atoms was proposed to describe the correlation of intermediate adsorption strengths and electronic structure quantificationally. Moreover, this work could provide some in-depth understanding of the excellent performance of single-atom catalysts and open some new perspectives for catalysts design.

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GB/T 7714 Liu, Dongyu , Liu, Ya , Zhou, Zhaohui et al. New Theoretical Strategy for the Correlation of Oxygen Evolution Performance and Metal Catalysts Adsorption at BiVO4 Surfaces [J]. | Journal of Physical Chemistry C , 2018 , 122 (44) : 25195-25203 .
MLA Liu, Dongyu et al. "New Theoretical Strategy for the Correlation of Oxygen Evolution Performance and Metal Catalysts Adsorption at BiVO4 Surfaces" . | Journal of Physical Chemistry C 122 . 44 (2018) : 25195-25203 .
APA Liu, Dongyu , Liu, Ya , Zhou, Zhaohui , Ding, Shujiang , Xia, Zhenhai , Li, Mingtao . New Theoretical Strategy for the Correlation of Oxygen Evolution Performance and Metal Catalysts Adsorption at BiVO4 Surfaces . | Journal of Physical Chemistry C , 2018 , 122 (44) , 25195-25203 .
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A new polysulfide blocker - poly(acrylic acid) modified separator for improved performance of lithium-sulfur battery EI SCIE Scopus
期刊论文 | 2018 , 563 , 277-283 | JOURNAL OF MEMBRANE SCIENCE
WoS CC Cited Count: 1
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Lithium-sulfur (Li-S) batteries gain great popularity due to its high theoretical energy density, low cost, and natural abundance of sulfur active elements, whereas, "shuttle effect" of soluble polysulfide seriously deteriorates their electrochemical performance, hindering their practical applications. Herein, we demonstrate a strategy that graft poly(acrylic acid) (PAA) on the surface of polypropylene (PP) separator to improve the electrochemical performance of Li-S batteries by impeding the "shuttle effect" of polysulfide. The PP grafted with PAA (PP-g-PAA) separator allows Li+ migration while rejects polysulfide anions by electrostatic repulsion. Consequently, this permselective separator restrains the polysulfide anions on the cathode side. In addition, the total reaction process of preparing PP-g-PAA separator is facile and low cost. Owing to the strong structure stability between PP and grafted PAA, a uniform and consistent blocking of the polysulfide shuttle during the charge-discharge process could be realized. An ultra-low decay value of 0.074% per cycle for the first 600 cycles is realized in this work. The electrochemical properties are significantly improved compared to the cell with PP separator. Such a permselective separator can be used in various electrodes and working conditions, which is promising for the construction of high performance batteries.

Keyword :

Permselective Polysulfide Separator Lithium-sulfur batteries Photografting

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GB/T 7714 Song, Shili , Shi, Lei , Lu, Shiyao et al. A new polysulfide blocker - poly(acrylic acid) modified separator for improved performance of lithium-sulfur battery [J]. | JOURNAL OF MEMBRANE SCIENCE , 2018 , 563 : 277-283 .
MLA Song, Shili et al. "A new polysulfide blocker - poly(acrylic acid) modified separator for improved performance of lithium-sulfur battery" . | JOURNAL OF MEMBRANE SCIENCE 563 (2018) : 277-283 .
APA Song, Shili , Shi, Lei , Lu, Shiyao , Pang, Yuanchao , Wang, Yuankun , Zhu, Min et al. A new polysulfide blocker - poly(acrylic acid) modified separator for improved performance of lithium-sulfur battery . | JOURNAL OF MEMBRANE SCIENCE , 2018 , 563 , 277-283 .
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